Phys. Rev. B 69, 134512 (2004) [7 pages]

Schottky anomaly in Nd2CuO4 observed by muon spin relaxation

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D. Baabe1 *, M. Hillberg1 , F. J. Litterst1, P. Adelmann2, and H.-H. Klauss1
1Institut für Metallphysik und Nukleare Festkörperphysik, TU Braunschweig, D-38106 Braunschweig, Germany
2Institut für Festkörperphysik, Forschungszentrum Karlsruhe, D-76021 Karlsruhe, Germany

Received 30 June 2003; revised 5 November 2003; published 20 April 2004

We report zero-field muon spin relaxation experiments on Nd2CuO4 focused on the low-temperature range for studying the Nd Schottky anomaly. In the magnetically ordered state we observed a significant increase and saturation of the muon spin precession frequency below T=15 K. A fit based on the temperature-dependent population of the Nd3+ Kramers ground-state doublet reveals a splitting of the doublet of Δ=4.2(6) K in good agreement with the work of Adelmann et al. [Phys. Rev. B 46, 3619 (1992)]. The same model was applied to account for the temperature dependence of the dynamic relaxation rate resulting in Δ=4.6(5) K. A quantitative evaluation of the temperature-dependent local magnetic field fluctuation rate is presented.


©2004 The American Physical Society

URL: http://link.aps.org/doi/10.1103/PhysRevB.69.134512
DOI: 10.1103/PhysRevB.69.134512
PACS: 74.72.Jt, 74.25.Ha, 76.75.+i

* Electronic address: d.baabe@tu-bs.de
Present address: TÜV Hannover/Sachsen-Anhalt e.V., D-70519 Hannover, Germany.

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