Phys. Rev. Lett. 84, 1411 - 1414 (2000)

Doubly Vibrationally Enhanced Four Wave Mixing: The Optical Analog to 2D NMR

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Wei Zhao and John C. Wright
Department of Chemistry, University of Wisconsin, Madison, Wisconsin 53706

Received 21 May 1999

We report the development of the four wave mixing vibrational analog to 2D NMR and demonstrate its spectral selectivity, sensitivity to the interactions causing mode coupling, and ability to spectrally resolve isotopic mixtures. The method discriminates against uncoupled vibrational modes and isolates the features that are associated with intra- or intermolecular interactions.

URL: http://link.aps.org/abstract/PRL/v84/p1411
DOI: 10.1103/PhysRevLett.84.1411
PACS: 33.40.+f

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Phys. Rev. Lett. 84, 1411 - 1414 (2000)

Doubly Vibrationally Enhanced Four Wave Mixing: The Optical Analog to 2D NMR

PRL Celebrates 50 Years